Twins' father 'studied poisons'
A police spokesman, Jean-Christophe Sauterel, said Matthias Kaspar Schepp also looked at websites listing "various means of suicide".
The six-year-old girls Alessia and Livia were reported missing by their mother on 30 January. She and Schepp were separated and had homes in Lausanne.
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Hide AdThe search for the twins spread to Corsica and southern Italy on Wednesday after authorities confirmed Schepp drove them to Marseilles and boarded a ferry for Corsica on 31 January.
Schepp, 43, apparently threw himself under a train in Cerignola, Italy, on 3 February.